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Anything Lupin III rules everything else. Anyone who hasn't seen Castle of Cagliostro really really needs to do so.
Inuyasha gets sneered at by hardcore animu types, but it's not all that bad at all in actuality. It's the Wonder Bread of anime, but hey, sometimes you just want to poke your frontal lobes out and enjoy a feel-good comedy/romance.
Trigun and Cowboy Bebop are also good choices for anime newcomers. The former is a lighthearted steampunk romp that sneaks an actual pathos-driven story in halfway through, the latter is essentially a very-well-done Lupin-knockoffs-in-space series, and both are on Adult Swim seemingly endlessly.
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